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Two Studies in Gas-Phase Ion Spectroscopy

Part of the Springer Theses Book Series

DOI: 10.1007/978-3-642-23129-2

ISBN: 978-3-642-23128-5

Publisher: Springer Berlin Heidelberg - Springer Journals

Oct 15, 2011

1 - 9 of 9 Chapters

LitStream

Chapter 1Introduction and Background Information

Simpson, Matthew J.

Pages: 1 –14

[The first part of this thesis reports and discusses results collected from an experiment designed to investigate the formation of ion pairs following the vacuum ultraviolet photoexcitation of a gas-phase molecule. The experiment is described in Chap. 2, and the results are discussed in Chaps....
LitStream

Chapter 2The Experiments

Simpson, Matthew J.

Pages: 15 –26

[Energy must be absorbed by a molecule in order for ion-pair dissociation to occur. Synchrotron radiation is ideal for such experiments because it provides a bright, monochromated and tunable energy source across the entire electromagnetic spectrum. Synchrotron radiation sources accelerate...
LitStream

Chapter 3Vacuum Ultraviolet Negative Photoion Spectroscopy of SF6, CF4 and SF5CF3

Simpson, Matthew J.

Pages: 27 –43

[This chapter focuses on the original data collected for trifluoromethyl sulphur pentafluoride (SF5CF3), however, the discussion extends to include the data also collected for the related molecules sulphur hexafluoride (SF6) and tetrafluoromethane (CF4). These results were collected in September...
LitStream

Chapter 4Vacuum Ultraviolet Negative Photoion Spectroscopy of CF3Cl, CF3Br and CF3I

Simpson, Matthew J.

Pages: 45 –63

[This chapter presents and analyses the data collected for trifluorochloromethane (CF3Cl), trifluorobromomethane (CF3Br) and trifluoroiodomethane (CF3I). This series of molecules will be referred to as the CF3X series, where X = Cl, Br or I, and the main aim of this study is to compare the data...
LitStream

Chapter 5Vacuum Ultraviolet Negative Photoion Spectroscopy of SF5Cl

Simpson, Matthew J.

Pages: 65 –74

[The experimental data for SF5Cl was collected in May 2008 on beamline 3.1 of the Daresbury synchrotron radiation source. Many thanks go to Dr David Shaw, Professor Colin Latimer, Dr Ken Dunn and Professor Richard Tuckett for providing their experimental expertise. This work has been accepted for...
LitStream

Chapter 6Vacuum Ultraviolet Negative Photoion Spectroscopy of Small Polyatomic Molecules

Simpson, Matthew J.

Pages: 75 –89

[A total of 24 small polyatomic molecules have been studied by the Chemical Physics groups in Birmingham and Belfast from 2005 to 2008 using VUV negative photoion spectroscopy:the data for SF5CF3, SF6 and CF4 were published in 2008 in the Journal of Chemical Physics , and updated here in Chap. 3;...
LitStream

Chapter 7The Reactions of CFn+ (n = 1–3) with C2H4, C2H3F, C2H2F2 and C2HF3

Simpson, Matthew J.

Pages: 91 –100

[This chapter reports a fundamental study which investigates on two fronts the effects of fluorination on the reactivity of small molecules. First, how increasing fluorine substitution in neutral ethene affects its reactivity, and second how using different fluorocarbon cation species in the...
LitStream

Chapter 8The Reactions of C2F4+ with C2H4, C2H3F, C2H2F2 and C2HF3

Simpson, Matthew J.

Pages: 101 –111

[This chapter continues the investigation on the effects of fluorination in ethene, but the reactant ion is now a fluorinated ethene itself, the tetrafluoroethene cation, C2F4+. In the original study of the reactions with CF+, CF2+ and CF3+ (Chap. 7) a new source gas was used, perfluoropropane...
LitStream

Chapter 9The Reactions of OH−, O−, CF3−, F−, and O−2 with C2H4, C2H3F, C2H2F2, C2HF3 and C2F4

Simpson, Matthew J.

Pages: 113 –134

[This chapter takes a new approach in the investigation of fluorination in ethene by looking at some anion-molecule reactions. The data presented were collected by Drs Richard Kennedy and Chris Mayhew many years ago. The raw data was given to me for a project which I started in the fourth year of...

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