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Molecular Conformation and Organic Photochemistry

Part of the Springer Theses Book Series

DOI: 10.1007/978-3-642-29381-8

ISBN: 978-3-642-29380-1

Publisher: Springer Berlin Heidelberg - Springer Journals

May 17, 2012

1 - 10 of 10 Chapters

LitStream

Introduction

Brogaard, Rasmus Y.

Pages: 3 –5

[The key difference between photochemistry and thermal chemistry is that the former is initiated in an excited electronic state. The topographies of the excited-state potential energy surfaces (PESs) are often fundamentally different from that of the ground state. This property makes...
LitStream

Aspects and Investigation of Photochemical Dynamics

Brogaard, Rasmus Y.

Pages: 7 –21

[This chapter starts by reviewing concepts that form a versatile means of describing nuclear motion and electronic structure changes during a photochemical reaction. This is followed by an introduction of a framework capable of describing how such ultrafast photodynamics can be probed...
LitStream

A Time-Resolved Probing Method: Photoionization

Brogaard, Rasmus Y.

Pages: 23 –33

[Seel and Domcke were the first to suggest the use of time-resolved photoionization experiments to investigate ultrafast molecular dynamics [1, 2]. Since then experimentalists all over the world have made numerous implementations of time-resolved photoionization experiments, of which this chapter...
LitStream

Simulation of Time-Resolved Photoionization Signals

Brogaard, Rasmus Y.

Pages: 37 –51

[In any scientific field there is a mutual benefit from the combination of theory and experiment in which progress in one discipline stimulates new efforts in the other. Thus, the pioneering theoretical work of Seel and Domcke lead to the birth of ultrafast time-resolved photoionization...
LitStream

Simulation: The Norrish Type-I Reaction in Acetone

Brogaard, Rasmus Y.

Pages: 53 –62

[In the following the theoretical framework introduced in the previous chapter is applied to a real case of ultrafast organic photodynamics: the Norrish Type-I reaction in acetone. Particular attention is payed to how the wave packet dynamics is expressed in the time-resolved photoionization...
LitStream

Experimental Setups

Brogaard, Rasmus Y.

Pages: 65 –73

[This chapter describes the experimental setups used to conduct the time-resolved photoionization experiments in the project. Some experiments were carried out in the Molecular Photonics Group at the Steacie Institute for Molecular Sciences, National Research Council Canada, in Ottawa and others...
LitStream

Paracyclophanes I: [2\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$$+$$\end{document}2]cycloaddition of Ethylenes

Brogaard, Rasmus Y.

Pages: 75 –88

[This chapter presents the first of two studies of photochemical reaction dynamics. The first section reviews the fundamental issue related to studying bimolecular reactions with fs time-resolution. This is followed by a presentation of the time-resolved investigation of the [2+2]cycloaddition...
LitStream

Paracyclophanes II: The Paternò-Büchi Reaction

Brogaard, Rasmus Y.

Pages: 89 –102

[This chapter presents the second study of a bimolecular photochemical reaction realized using the [2.2] paracyclophane scaffold. The reaction, a cycloaddition between a photoexcited carbonyl group and an alkene to form a four-membered cyclic ether (oxetane), is named the Paternò-Büchi (PB)...
LitStream

Probing Structural Dynamics by Interaction Between Chromophores

Brogaard, Rasmus Y.

Pages: 103 –114

[This chapter deals with the experimental results published in Ref. IV in which structural dynamics in the radical cation of 1,3-dibromopropane (DBP) was probed by exploiting the interaction between the bromine atoms. As such, this experiment illustrates a simpler, although not as general, way of...
LitStream

Summarizing Discussion

Brogaard, Rasmus Y.

Pages: 117 –120

[For most chemists the concept of the ground state reaction path as being the minimum-energy path from reactants to products along the potential energy surface (PES) is an essential part of their educational upbringing. Induced by optical excitations, photochemical reactions involve excited-state...

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