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Transformation of Carbon Dioxide to Formic Acid and Methanol

Part of the SpringerBriefs in Molecular Science Book Series

DOI: 10.1007/978-981-10-3250-9

ISBN: 978-981-10-3249-3

Publisher: Springer Singapore - Springer Journals

Oct 28, 2017

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Chapter 1Introduction

Wang, Wan-Hui; Feng, Xiujuan; Bao, Ming

Pages: 1 –6

[ Huge amount of carbon dioxide emission poses a serious threat to our environmental and biological systems. Development of sustainable energy system based on CO2 is highly desired. This chapter briefly introduces the approaches of CO2 activation and transformation, and emphasizes CO2 reduction...
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Chapter 2Transformation of CO2 to Formic Acid or Formate with Homogeneous Catalysts

Wang, Wan-Hui; Feng, Xiujuan; Bao, Ming

Pages: 7 –42

[ Homogeneous hydrogenation of carbon dioxide to formic acid or formate has attracted much attention due to its high performance. Various metals including noble metals and nonprecious metals combined with different ligands have been investigated. The catalytic mechanism and catalyst design...
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Chapter 3Transformation of CO2 to Formic Acid or Formate Over Heterogeneous Catalysts

Wang, Wan-Hui; Feng, Xiujuan; Bao, Ming

Pages: 43 –52

[Although heterogeneously catalytic CO2 hydrogenation to formate was discovered 100 years ago, only recently important progress has been achieved. This chapter covers the most recent reported heterogeneous catalysts using Ni, Pd, Ru, Ir, and Au. The catalyst design and catalytic performance are...
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Chapter 4Transformation of CO2 to Methanol with Homogeneous Catalysts

Wang, Wan-Hui; Feng, Xiujuan; Bao, Ming

Pages: 53 –87

[ Homogeneous hydrogenation of carbon dioxide to methanol is highly challenging. Only a few examples using hydrogen as reductant have been reported. Considerable studies employ borane or silane as a reductant. Although these hydrogen sources are expensive, these studies have achieved higher...
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Chapter 5Transformation of CO2 to Methanol Over Heterogeneous Catalysts

Wang, Wan-Hui; Feng, Xiujuan; Bao, Ming

Pages: 89 –119

[ Hydrogenation of CO2 to methanol over heterogeneous catalysts usually requires hash conditions. Various heterogeneous catalysts based on Cu, Pd, Ni, Ag, Au, In, and other metals have been recently developed and investigated. Cu doped by other metals or metal oxides are the preferred selection....
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Chapter 6Conclusions and Outlook

Wang, Wan-Hui; Feng, Xiujuan; Bao, Ming

Pages: 121 –123

[ In this chapter, we summarize all the homogeneous and heterogeneous transformation of CO2 to formate/formic acid and methanol. The important factors such as solvent, additive, metal, ligand, and hydrogen source that influence the reaction performance are discussed.]

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